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有色金属(冶炼部分):2025,(1):110-118
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基于COMSOL+PHREEQC耦合数值模拟的浸出实验研究——以内蒙古某铀矿浸出工艺试验为例
张传飞1, 何斌1, 骆桂君2, 刘金辉3, 许影4, 陈梅芳4
(1.中核内蒙古矿业有限公司;2.中南大学;3.东华理工大学;4.核工业北京化工冶金研究院)
Leaching Test Study Based on COMSOL+PHREEQC Coupled Numerical Simulation:A Case Study of Uranium Leaching Process in Inner Mongolia
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投稿时间:2024-07-17     修订日期:2024-10-07     录用日期:2024-10-08     网络发布日期:2025-02-18
中文摘要: 室内浸出工艺实验是联系科研和工业生产的必要环节,针对可地浸砂岩型铀矿浸出工艺室内实验条件与工业生产条件不同、物理实验组数多、矿岩采取困难等问题,提出了1套基于COMSOL+PHREEQC耦合的地浸采铀柱浸数值模拟模型构建方法,并以内蒙古某铀矿浸出室内试验为例,开展了物理实验与数值模拟实验对比研究。结果表明:采用基于COMSOL+PHREEQC耦合的数值模拟法,在酸法浸出室内柱浸实验模拟方面,具有良好的可行性;相同压力条件下,pH值、U、Fe3+、Ca2+ 、SO42-等溶出组分的浸出规律基本一致,峰值出现的时间相对较吻合;不同压力条件下,数值模拟模型的结果符合压力调节情况下的一般规律;所建数值模拟模型在U、Ca2+浓度峰值大小方面尚存在差异,需要进一步完善模拟模型。
Abstract:The indoor leaching process experiment is a necessary link between scientific research and industrial production. In view of the differences between the indoor experimental conditions and industrial production conditions for the leaching process of in-situ leachable sandstone-type uranium deposits, the large number of physical experiment groups, and the difficulty of mining and rock sampling, a set of numerical simulation model construction methods for in-situ leachable uranium mining column leaching based on the coupling of COMSOL and PHREEQC is proposed. Taking the indoor leaching experiment of a certain uranium deposit in Inner Mongolia as an example, a comparative study of physical experiments and numerical simulation experiments was carried out. The results show that the numerical simulation method based on the coupling of COMSOL and PHREEQC has good feasibility in the simulation of acid leaching indoor column leaching experiments. Under the same pressure conditions, the leaching rules of dissolved components such as pH value, U, Fe3+, Ca2+, and SO42- are basically consistent, and the time of peak occurrence is relatively consistent. Under different pressure conditions, the results of the numerical simulation model conform to the general rules under pressure adjustment. There are still differences in the peak values of U and Ca2+ concentrations in the constructed numerical simulation model, which needs further improvement of the simulation model.
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基金项目:中国铀业自主科研项目(CNUC-YF2021)
引用文本:
张传飞,何斌,骆桂君,刘金辉,许影,陈梅芳.基于COMSOL+PHREEQC耦合数值模拟的浸出实验研究——以内蒙古某铀矿浸出工艺试验为例[J].有色金属(冶炼部分),2025(1):110-118.
ZHANG Chuan-fei,HE bin,LUO Guijun,LIU Jinhui,XU Ying,CHEN Meifang.Leaching Test Study Based on COMSOL+PHREEQC Coupled Numerical Simulation:A Case Study of Uranium Leaching Process in Inner Mongolia[J].Nonferrous Metals (Extractive Metallurgy),2025(1):110-118.

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