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有色金属(冶炼部分):2023,(10):149-157
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煤炭矿区排矸场表层土壤重金属污染研究
张肖萌1, 郭巧玲1, 杨云松2,2, 代彬1
(1.东华理工大学 水资源与环境工程学院;2.南昌工学院 经济与管理学院)
Study on Heavy Metal Pollution in Topsoil of Gangue Field in Coal Mining Area
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投稿时间:2023-05-24     修订日期:2023-06-01     录用日期:2023-06-05     网络发布日期:2023-09-04
中文摘要: 采用填埋覆土的方式对煤矸石进行处理,在沉陷区沟壑地带分层充填矸石,使沟地变为平地,对环境保护有重要意义。神府东胜煤田的大多数煤矿现已基本采用填埋覆土的方式对煤矸石进行处理。以神府东胜煤田中某排矸场为研究对象,分析了排矸场表层土壤(地表及-1 m处)中As、Cd、Cr、Cu、Mn、Ni、Pb和Zn含量的空间分布特征及土壤中重金属的赋存形态。研究表明,排矸场中As、Cd、Cr、Cu、Pb、Zn含量超过该地区的土壤背景值,对当地的土壤环境造成了一定的污染;排矸场土壤中As、Cd、Cr、Cu、Mn、Ni、Pb在-1 m处的含量高于表层土壤,并且排矸场中-1 m处土壤的8种重金属元素的含量都高于对照区土壤重金属含量;排矸场中Cd、Cr、Cu、Ni残渣态占比最大,As可氧化态占比最大,Mn、Zn、Pb可交换态和可还原态占比较大,Mn、Zn、Pb以更不稳定的形态存在,对生态环境影响较大。
Abstract:It is of great significance for environmental protection to treat coal gangue by landfilling and covering with soil, and to fill the subsidence area with gangue in layers to make the gully land flat. At present, most coal mines in Shenfu Dongsheng Coalfield have treated coal gangue by the way of landfilling. Applying a gangue dump in the Shenfu Dongsheng Coalfield as the research object to analyze the spatial distribution characteristics of As, Cd, Cr, Cu, Mn, Ni, Pb, and Zn contents in the surface soil (surface and -1 m away) of the waste dump, as well as the occurrence forms of heavy metals in the soil. The results show that the contents of As, Cd, Cr, Cu, Pb and Zn in gangue dumping field exceed the soil background value of this area, causing pollution to the local soil environment to some extent. The contents of As, Cd, Cr, Cu, Mn, Ni and Pb in the soil at -1 m are higher than that in the surface soil, and the contents of eight heavy metals in the soil at -1 m are higher than that in the control area. In gangue discharge field, the residuals of Cd, Cr, Cu and Ni account for the largest proportion; the oxidizable states of As account for the largest proportion; The exchangeable and reducible states of Mn, Zn and Pb account for a large proportion; Mn, Zn and Pb exist in more unstable forms, which have a great impact on the ecological environment.
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基金项目:国家自然科学基金资助项目(42162021);东华理工大学博士基金资助项目(DHBK2019093);江西省水利科技重点项目(202325ZDKT01)
引用文本:
张肖萌,郭巧玲,杨云松,代彬.煤炭矿区排矸场表层土壤重金属污染研究[J].有色金属(冶炼部分),2023(10):149-157.
ZHANG Xiaomeng,GUO Qiaoling,YANG Yunsong,DAI Bing.Study on Heavy Metal Pollution in Topsoil of Gangue Field in Coal Mining Area[J].Nonferrous Metals (Extractive Metallurgy),2023(10):149-157.

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