本文已被:浏览 1819次 下载 1935次
投稿时间:2022-12-03 修订日期:2022-12-07 录用日期:2022-12-12 网络发布日期:2023-03-17
投稿时间:2022-12-03 修订日期:2022-12-07 录用日期:2022-12-12 网络发布日期:2023-03-17
中文摘要: 以某铅锌尾矿库周边农用地土壤和底泥为研究对象,运用富集因子指数法、潜在生态风险指数法和GIS地统计分析土壤和底泥Tl的污染水平和分布特征,并采用蒙特卡罗模拟的健康风险模型探析研究区土壤Tl对人体的健康风险。结果表明,研究区土壤和底泥Tl含量均值分别为0.54和0.77 mg/kg。富集因子指数表明,土壤Tl富集因子指数均值为0.77,以无富集(EF<1)为主,占比75%;底泥Tl富集因子指数均值为1.10,均为轻度富集(1≤EF<3)。潜在生态风险指数表明,土壤Tl潜在生态风险指数均值为30.9,以轻微生态风险(E_r^i<40)为主,占比75%;底泥Tl潜在生态风险指数均值为43.9,以中等生态风险(40≤E_r^i<80)为主,占比75%。空间分析表明,铅锌尾矿库下游底泥和距尾矿库150 m内的土壤Tl污染程度相对较高,说明受尾矿库堆存长期影响。健康风险表明,土壤Tl对儿童和成人非致癌健康风险可忽略,非致癌健康风险指数均值分别为0.038 2和0.003 27,土壤Tl含量和土壤颗粒摄入速率的敏感度最大,应作为优先控制要素。
Abstract:The enrichment factor index method, Hakanson index method and GIS geostatistical analysis were used to analyze the pollution level and distribution characteristics of Tl in soil and sediment around one typical lead-zinc tailings. The health risk of Tl in soil to human was analyzed by health risk assessment model employed by Monte Carlo simulation. The results show that average content of Tl in soil and sediment is 0.54 and 0.77 mg/kg respectively. Average enrichment factor index of Tl in soil is 0.77, which 75% of the samples are un-enrichment (EF<1), however, average enrichment factor index of Tl in sediment is 1.10, which 100% of the samples are slight enrichment (1≤EF<3). Average Hakanson index of Tl in soil is 30.9, which 75% of the samples are slight ecological risk (E_r^i<40), however, average Hakanson index of Tl in sediment is 43.9, which 75% of the samples are medium ecological risk (40≤E_r^i<80). The spatial analysis shows that Tl pollution in the sediment downstream of the lead-zinc tailings pond and within 150 m in soil from the tailings pond is relatively high, which indicates that it is affected by tailing pond storage for a long time. Health risk assessment of Tl shows that non-carcinogenic health risks of children and adults can be ignored, which average non-carcinogenic health risk indexes are 0.038 2 and 0.003 27 respectively. Content of Tl in soil and ingestion rate of soil particle are the most sensitive factors, which should be taken as the priority control factors.
文章编号: 中图分类号: 文献标志码:
基金项目:重庆市生态环境局项目(2021-111);重庆市科学技术局绩效激励引导专项(cstc2021jxj120002)
| 作者 | 单位 | |
| 马杰 | 重庆市生态环境监测中心 农村生态与土壤监测技术研究中心 | pony312@qq.com |
| 孙静 | 重庆市生态环境监测中心 农村生态与土壤监测技术研究中心 | |
| 蒋月* | 重庆市生态环境监测中心 农村生态与土壤监测技术研究中心 | 550783895@qq.com |
| 陈召沪 | 重庆市生态环境监测中心 农村生态与土壤监测技术研究中心 | |
| 刘萍 | 重庆市生态环境监测中心 农村生态与土壤监测技术研究中心 |
引用文本:
马杰,孙静,蒋月,陈召沪,刘萍.某铅锌尾矿库周边土壤和底泥重金属铊污染特征及健康风险评估[J].有色金属(冶炼部分),2023(4):140-147.
MA Jie,SUN Jing,JIANG Yue,CHEN Zhao-hu,LIU Ping.Pollution Characteristics and Health Risk Assessment of Thallium in Soils and Sediments of a Lead-Zinc Tailings[J].Nonferrous Metals (Extractive Metallurgy),2023(4):140-147.
马杰,孙静,蒋月,陈召沪,刘萍.某铅锌尾矿库周边土壤和底泥重金属铊污染特征及健康风险评估[J].有色金属(冶炼部分),2023(4):140-147.
MA Jie,SUN Jing,JIANG Yue,CHEN Zhao-hu,LIU Ping.Pollution Characteristics and Health Risk Assessment of Thallium in Soils and Sediments of a Lead-Zinc Tailings[J].Nonferrous Metals (Extractive Metallurgy),2023(4):140-147.

关注微信公众号